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FDPHOTOC15:Comparison of Self-Assembled and Micelle Encapsulated QD Chemosensor Constructs for Biological Sensing

20 July, 2015 - 00:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00093A, PaperDaniel G. Nocera, Christopher M. Lemon
Whereas a variety of covalent conjugation strategies have been utilized to prepare quantum dot (QD)-based nanosensors, supramolecular approaches of self-assembly have been underexplored. A major advantage of self-assembly is the...
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Determination of the kinetics underlying the pKa shift for 2-aminoanthracenium cation binding with cucurbit[7]uril

17 July, 2015 - 23:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00095E, PaperOpen Access Open Access Creative Commons Licence&nbsp This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Cornelia Bohne, Suma S. Thomas
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FD2015-Single Molecule Microscopy: Polarization Effects in Lattice-STED Microscopy

15 July, 2015 - 23:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00092K, PaperBin Yang, Chia-Yi FANG, Huan-Cheng Chang, Francois TREUSSART, Jean-Baptiste Trebbia, Brahim Lounis
Massive parallelization of STED-like nanoscopies is now achievable using well-designed optical lattices for state depletion. Yet, only the lattice intensity distribution was considered for the description of the super-resolved point...
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Highly Optimized CO2 Capture by Inexpensive Nanoporous Covalent Organic Polymers and Their Amine Composites

15 July, 2015 - 23:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00099H, PaperHasmukh A Patel, Cafer Yavuz
Carbon dioxide (CO2) storage and utilization requires effective capture strategies that limit energy penalties. Polyethylenimine (PEI)-impregnated covalent organic polymers (COPs) with high CO2 adsorption capacity are successfully prepared in this...
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FDPHOTOC15: Photoelectrochemical Properties of Porphyrin Dyes with a Molecular Dipole in the Linker

13 July, 2015 - 22:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00082C, PaperKen T. Ngo, Jonathan Rochford, Hao Fan, Alberto Batarseh, Keyur Chitre, Sylvie Rangan, Robert A. Bartynski, Elena Galoppini
The electronic properties of three porphyrin-bridge-anchor photosensitizers are reported with (1a,e and 3a,e) or without (2a,e) an intramolecular dipole in the bridge. The presence and orientation of the bridge dipole...
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FDCDU15 - Carbon Dioxide Utilisation: Improving the efficiency of electrochemical CO2 reduction using immobilized manganese complexes

9 July, 2015 - 21:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00071H, PaperJames J Walsh, Charlotte L Smith, Gaia Neri, George F. S. Whitehead, Craig M Robertson, Alexander J. Cowan
Immobilization of [Mn(bpy)(CO)3Br], (1) and [Mn(bpy(tBu)2)(CO)3Br] (2, where (bpy(tBu)2) = 4,4'-di-tert-butyl-2,2'-bipyridine) in Nafion/multi-walled carbon nanotube films (MWCNT) on glassy carbon yielded highly active electrodes for the reduction of CO2 to...
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Electrocatalytic conversion of CO2 to produce solar fuels in electrolyte or electrolyte-less configurations of PEC cells

9 July, 2015 - 21:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00069F, PaperGabriele Centi, Claudio Ampelli, Chiara Genovese, Bhanu Chandra Marepally, Georgia Papanikolaou, Siglinda Perathoner
The electrocatalytic reduction of CO2 is studied on a series of electrodes (based on Cu, Co, Fe and Pt metal nanoparticles deposited on carbon nanotubes or carbon black and then...
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FDCDU15 - Investigating public perceptions of Carbon Dioxide Utilisation (CDU) technology: a mixed methods study

9 July, 2015 - 21:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00063G, PaperChristopher Jones, Daphne Kaklamanou, William Stuttard, Rebecca Radford, Jane Burley
Carbon Dioxide Utilisation (CDU) technologies hold promise for helping to limit atmospheric releases of CO2 while generating saleable products. However, while there is growing investment in the research and development...
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FDCDU15 - Carbon Dioxide Utilisation: Exploiting CO2 vibrational excitation to achieve an energy efficient route for CO2 based artificial fuels

9 July, 2015 - 21:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00045A, PaperGerard van Rooij, Dirk van den Bekerom, Niek den Harder, Teofil Minea, Giel Berden, Waldo Bongers, Richard Engeln, Martijn Graswinckel, Erwin Zoethout, Mauritius C.M. van de Sanden
The strong non-equilibrium conditions provided by the plasma phase offer the opportunity to beat traditional thermal process energy efficiencies via preferential excitation of molecular vibrations. Simple molecular physics considerations are...
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FDPHOTOC15: Water oxidation catalysis upon evolution of molecular Co(III) cubanes in aqueous media

7 July, 2015 - 21:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00076A, PaperAndrea Sartorel, Andrea Genoni, giuseppina LaGanga, Andrea Volpe, Fausto Puntoriero, Marilena Di Valentin, Marcella Bonchio, Mirco Natali
The increasing global energy demand has stimulated great, recent efforts in investigating new solutions for artificial photosynthesis, a potential source of clean and renewable solar fuels. In particular, according to...
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Single Molecule Microscopy: An integrated system for optical and electrical detection of single molecules/particles inside a solid-state nanopore

7 July, 2015 - 21:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00060B, PaperXin Shi, Rui Gao, Yi-Lun Ying, Wei Si, Yunfei Chen, Yi-Tao Long
Nanopore techniques have proven to be conspicuous tools for single-molecule detection. The combination of optical detection and ion current measurement enables the new possibility of parallel readout of multiple nanopores...
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FDPHOTOC15: Synthesis and Strong Photooxidation Power of a Supramolecular Hybrid comprising a Polyoxometalate and Ru(II) Polypyridyl Complex with Zinc(II)

7 July, 2015 - 21:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00080G, PaperKenji Ohashi, Hiroyuki Takeda, Kazuhide Koike, Osamu Ishitani
A novel method for constructing supramolecular hybrids composed of polyoxometalates and photofunctional metal complexes was developed. A Ru(II) complex with phosphonate groups (RuP) strongly interacted with Zn(II) to afford a...
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FDPHOTOC15: Spatiotemporal Control Over the Co-Conformational Switching in pH-Responsive Flavylium-Based Multistate Pseudorotaxanes

7 July, 2015 - 21:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00078E, PaperAna Marta Diniz, Nuno Basilio, Hugo Cruz, Fernando Pina, A. Jorge Parola
A multistate molecular dyad containing flavylium and viologen units was synthesized and the pH dependent thermodynamics of the network completely characterized by a variety of spectroscopic techniques such as NMR,...
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Ruthenium Catalysts for Water Oxidation Involving Tetradentate Polypyridine-type Ligands

7 July, 2015 - 21:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00051C, PaperRandolph P Thummel, Lianpeng Tong, Ruifa Zong, Rongwei Zhou, Nattawut Kaveevivitchai, Gang Zhang
A series of RuII complexes that behave as water oxidation catalysts were prepared involving a tetradentate equatorial ligand and two 4-substituted pyridines as the axial ligands. Two of these complexes...
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Environmental potential of carbon dioxide utilization in the polyurethane supply chain

5 July, 2015 - 20:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00067J, PaperNiklas von der Assen, Andre Sternberg, Arne Katelhon, Andre Bardow
Potential environmental benefits have been identified for the utilization of carbon dioxide (CO2) as feedstock for polyurethanes (PUR). CO2 can be utilized in the PUR supply chain in a wide...
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Extraction of Mg(OH)2 from Mg silicate minerals with NaOH assisted with H2O: implications for CO2 capture from exhaust flue gas

3 July, 2015 - 20:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00047E, PaperSilvia Madeddu, Michael Priestnall, Eric Godoy, Ramachandran Vasant Kumar, Sugat Raymahasay, Michael Evans, Ruofan Wang, Seabelo Manenye, Hajime Kinoshita
The utilisation of Mg(OH)2 to capture exhaust CO2 has been hindered by the limited availability of brucite, Mg(OH)2 mineral in natural deposits. Our previous study demonstrated that Mg(OH)2 can be...
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Photoswitchable stable charge-distributed states in a new Cobalt complex exhibiting photo-induced valence tautomerism

1 July, 2015 - 19:54
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00088B, PaperMichael Slota, Marian Blankenhorn, Eric Heintze, Minh Vu, Ralph Hubner, Lapo Bogani
We report the synthesis, magnetic and photomagnetic behaviour of a novel valence tautomeric cobalt complex, [Co(3,5-dbbq)2([small mu ]-bpym)] (1) (3,5-dbbq=3,5-di-tert-butyl-1,2-benzoquinone and [small mu ]-bpym=2,2'-bipyrimidine). The synthesis is performed by reacting Co2(CO)8 and [small mu ]-bpym in...
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FDPHOTOC15: Parameters influencing the photo-induced electron transfer from tryptophan containing peptides to a RuII complex: a systematic study

29 June, 2015 - 19:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00059A, PaperKevin Garnir, Sandra Estalayo-Adrian, Remy Lartia, Julien De Winter, Eric Defrancq, Mathieu Surin, Vincent Lemaur, Pascal Gerbaux, Cecile Moucheron
Ruthenium (II) polyazaaromatic complexes gained interest in the last decades as biomolecular tools especially in the development of new phototherapeutic agents. Those light emissive Ru complexes based on pi-deficient ligands...
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FDPHOTOC15: Solvent tuned single molecule dual emission in protic solvents: effect of polarity and H-bonding

29 June, 2015 - 19:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00054H, PaperSylviane Chevreux, Clemence Allain, Liam Wilbraham, Keitaro Nakatani, Patrice Jacques, Ilaria Ciofini, Gilles LEMERCIER
Phen-PENMe2 has been recently proposed as a promising new molecule displaying solvent-tuned dual emission highlighting an original and newly-described OPICT ("Orthogonal [small pi]-Orbital Planar Intramolecular Charge Transfer") model. Study was continued...
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FDCDU15 - Carbon Dioxide Utilisation: A framework for the analysis of the security of supply of utilising Carbon Dioxide as a chemical feedstock

29 June, 2015 - 19:17
Faraday Discuss., 2015, Accepted Manuscript
DOI: 10.1039/C5FD00038F, PaperEric Fraga, Melvin Ng
Recent developments in catalysts have enhanced the potential for the utilisation of carbon dioxide as a chemical feedstock. Appropriate catalysts make possible and/or energy efficient a range of chemical pathways...
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