Chem. Soc. Rev.

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Template-directed synthesis of metal-organic materials

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5444-5455
DOI: 10.1039/C4CS00075G, Tutorial ReviewZhenjie Zhang, Michael J. Zaworotko
This tutorial review details the emergence of template-directed synthesis of metal-organic materials (MOMs) with emphasis upon reports of MOMs in which the template is retained, template@MOMs, and structurally characterized.
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Cation exchange at the secondary building units of metal-organic frameworks

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5456-5467
DOI: 10.1039/C4CS00002A, Tutorial ReviewOpen Access Open Access Creative Commons Licence&nbsp This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.C. K. Brozek, M. Dinca
This review examines the governing factors of cation exchange at the secondary building units of MOFs and reviews its applications.
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Application of electronic circular dichroism in the study of supramolecular systems

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5211-5233
DOI: 10.1039/C4CS00104D, Tutorial ReviewGennaro Pescitelli, Lorenzo Di Bari, Nina Berova
Electronic circular dichroism (ECD) is a choice technique for the analysis of chiral supramolecular systems, including their detection, determination of thermodynamic and kinetic quantities, and structural elucidation.
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Supramolecular templating of hierarchically porous metal-organic frameworks

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5431-5443
DOI: 10.1039/C4CS00127C, Tutorial ReviewDarren Bradshaw, Samir El-Hankari, Lucia Lupica-Spagnolo
This tutorial review summarises recent advances in the soft templating of metal-organic frameworks with hierarchical porosity across the micro- and mesoporous regimes.
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Structuring of metal-organic frameworks at the mesoscopic/macroscopic scale

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5700-5734
DOI: 10.1039/C4CS00106K, Review ArticleShuhei Furukawa, Julien Reboul, Stephane Diring, Kenji Sumida, Susumu Kitagawa
This review conceptually categorizes the available synthetic methodologies for structuring of MOFs in the mesoscopic and macroscopic scales.
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Design and synthesis of organic-inorganic hybrid capsules for biotechnological applications

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5192-5210
DOI: 10.1039/C4CS00108G, Tutorial ReviewJiafu Shi, Yanjun Jiang, Xiaoli Wang, Hong Wu, Dong Yang, Fusheng Pan, Yanlei Su, Zhongyi Jiang
The design, synthesis and biotechnological applications of organic-inorganic hybrid capsules are briefly reviewed and selectively highlighted.
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Reactions of metallocarbenes derived from N-sulfonyl-1,2,3-triazoles

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5151-5162
DOI: 10.1039/C4CS00072B, Tutorial ReviewHuw M. L. Davies, Joshua S. Alford
Metal-stabilized carbenes derived from N-sulfonyl triazoles have become broadly useful reactive intermediates for organic synthesis.
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Challenges in reduction of dinitrogen by proton and electron transfer

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5183-5191
DOI: 10.1039/C4CS00085D, Tutorial ReviewCornelis J. M. van der Ham, Marc T. M. Koper, Dennis G. H. Hetterscheid
Catalytic reduction of dinitrogen with protons and electrons is a very challenging alternative to the energy expensive Haber-Bosch reaction.
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MOF positioning technology and device fabrication

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5513-5560
DOI: 10.1039/C4CS00089G, Review ArticlePaolo Falcaro, Raffaele Ricco, Cara M. Doherty, Kang Liang, Anita J. Hill, Mark J. Styles
Methods for permanent localisation, dynamic localisation and spatial control of functional materials within MOF crystals are critical for the development of miniaturised MOF-based devices for a number of technological applications.
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MOF-based electronic and opto-electronic devices

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5994-6010
DOI: 10.1039/C4CS00096J, Review ArticleV. Stavila, A. A. Talin, M. D. Allendorf
Emergent properties resulting from the ordered structure and synthetic versatility of nanoporous metal-organic frameworks offer exciting possibilities for electronic devices.
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Harnessing the chemistry of graphene oxide

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5288-5301
DOI: 10.1039/C4CS00060A, Review ArticleDaniel R. Dreyer, Alexander D. Todd, Christopher W. Bielawski
The chemistry of graphene oxide is revisited, and includes an update on recent developments and potential applications.
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Amyloid-based nanosensors and nanodevices

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5326-5345
DOI: 10.1039/C4CS00082J, Review ArticleCharlotte A. E. Hauser, Sebastian Maurer-Stroh, Ivo C. Martins
Exploring amyloid-like peptides and proteins for applications in nanotechnology will open up new strategies for potential applications, such as biomedical therapies, biosensing, disease diagnostics, biomarker screening, bioimaging and monitoring.
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Nanochemistry-derived Bi2WO6 nanostructures: towards production of sustainable chemicals and fuels induced by visible light

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5276-5287
DOI: 10.1039/C4CS00056K, Review ArticleNan Zhang, Rosaria Ciriminna, Mario Pagliaro, Yi-Jun Xu
The advances of Bi2WO6 nanostructures utilized in photocatalytic organic synthesis and fuel production under visible light are discussed and prospected.
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High-throughput computational screening of metal-organic frameworks

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5735-5749
DOI: 10.1039/C4CS00070F, Review ArticleYamil J. Colon, Randall Q. Snurr
High-throughput computational screening of MOFs allows identification of promising candidates, new structure-property relationships, and performance limits.
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Metal-organic frameworks for artificial photosynthesis and photocatalysis

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5982-5993
DOI: 10.1039/C4CS00103F, Review ArticleTeng Zhang, Wenbin Lin
This article reviews the latest progress in light-harvesting, organic photocatalysis, proton and CO2 reduction, and water oxidation using MOFs.
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Low-molecular-mass gels responding to ultrasound and mechanical stress: towards self-healing materials

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5346-5371
DOI: 10.1039/C4CS00066H, Review ArticleXudong Yu, Liming Chen, Mingming Zhang, Tao Yi
Ultrasound and mechanical stress-driven/-responsive LMOGs, which are used extensively to construct self-healing materials with reversibility, are highlighted.
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Mesosilica materials and organic pollutant adsorption: part B removal from aqueous solution

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5173-5182
DOI: 10.1039/C3CS60095E, Tutorial ReviewL. T. Gibson
This tutorial review will focus on the removal of organic pollutants from the aqueous phase by mesoporous silica.
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Mesosilica materials and organic pollutant adsorption: part A removal from air

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5163-5172
DOI: 10.1039/C3CS60096C, Tutorial ReviewL. T. Gibson
This tutorial review focuses on the application of mesoporous silica materials, primarily MCM-41 and SBA-15, for the removal of organic pollutants in the vapour phase.
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Substitution reactions in metal-organic frameworks and metal-organic polyhedra

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5952-5981
DOI: 10.1039/C4CS00033A, Review ArticleYi Han, Jian-Rong Li, Yabo Xie, Guangsheng Guo
This review summarizes the advances in the study of substitution reactions in metal-organic frameworks (MOFs) and metal-organic polyhedra (MOPs).
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Post-synthetic metalation of metal-organic frameworks

25 July, 2014 - 10:17

Chem. Soc. Rev., 2014, 43,5933-5951
DOI: 10.1039/C4CS00076E, Review ArticleJack D. Evans, Christopher J. Sumby, Christian J. Doonan
Post-synthetic metalation (PSMet) offers expansive scope for a targeted approach to tailoring the properties of MOFs.
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