Chem. Soc. Rev.

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Recent advances in the synthesis of pyrroles by multicomponent reactions

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C3CS60015G, Review ArticleVeronica Estevez, Mercedes Villacampa, J. Carlos Menendez
Efficient and environmentally attractive access to pyrroles can be gained by use of multicomponent reactions.
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Recent advances in porous polyoxometalate-based metal-organic framework materials

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C3CS60404G, Review ArticleDong-Ying Du, Jun-Sheng Qin, Shun-Li Li, Zhong-Min Su, Ya-Qian Lan
POM-based MOF materials, which combine the advantages of both POMs and MOFs, have received increasing attention. In this review, we present the recent developments in porous POM-based MOF materials for the first time, including their classification, synthesis strategies and applications, especially in the field of catalysis.
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Chemical applications carried out by local pair natural orbital based coupled-cluster methods

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C4CS00050A, Review ArticleManuel Sparta, Frank Neese
Local pair natural orbital coupled-cluster methods are suitable for accurate assessment of the energies of large molecular and supramolecular systems.
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Laboratory spectroscopy of astrophysically relevant carbon species

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C4CS00049H, Review ArticleLindsay N. Zack, John P. Maier
Laboratory spectroscopic methods developed to measure the electronic spectra of astrophysically relevant carbon containing molecules, including radicals and ions, are discussed.
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Progress in allene chemistry

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,2886-2887
DOI: 10.1039/C4CS90020K, EditorialBenito Alcaide, Pedro Almendros
Guest editors Benito Alcaide and Pedro Almendros introduce the Progress in allene chemistry themed issue of Chemical Society Reviews.
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Mechanistic insights into the gold chemistry of allenes

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,2941-2955
DOI: 10.1039/C3CS60441A, Tutorial ReviewWeibo Yang, A. Stephen K. Hashmi
In the last few years numerous new gold-catalysed reactions of allenes have been developed. The current mechanistic knowledge about different versatile reaction types like cycloadditions, hydroarylations, hydroalkoxylations and additions of carbonyl derivatives is based on experimental evidence and computational studies.
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Synthesis and properties of long [n]cumulenes (n [greater-than-or-equal] 5)

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,3184-3203
DOI: 10.1039/C4CS00022F, Review ArticleJohanna A. Januszewski, Rik R. Tykwinski
This review highlights the synthesis and reactivity of longer [n]cumulenes (n [greater-than-or-equal] 5) and summarizes their electronic and structural properties.
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Metal complexes designed to bind to amyloid-[small beta] for the diagnosis and treatment of Alzheimer's disease

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C4CS00026A, Review ArticleDavid J. Hayne, SinChun Lim, Paul S. Donnelly
The use radioactive copper and technetium complexes as amyloid imaging agents, the use of luminescent metal complexes as non-conventional probes of amyloid formation and the potential of metal complexes to be inhibitors of amyloid toxicity are discussed.
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Zeolites as catalysts in oil refining

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C3CS60394F, Tutorial ReviewAna Primo, Hermenegildo Garcia
This tutorial review describes the general properties of zeolites and their prevalent role as heterogeneous catalysts in oil refining.
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Protein film photoelectrochemistry of the water oxidation enzyme photosystem II

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C4CS00031E, Tutorial ReviewMasaru Kato, Jenny Z. Zhang, Nicholas Paul, Erwin Reisner
This review describes key functions of the water oxidation enzyme photosystem II, protein film photoelectrochemistry of photosystem II and bio-inspired photoelectrochemical water oxidation systems.
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Silver and platinum-catalysed addition of O-H and N-H bonds to allenes

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,3164-3183
DOI: 10.1039/C3CS60408J, Review ArticleMaria Paz Munoz
Silver and platinum-catalysed reactions of allenes with oxygen and nitrogen nucleophiles are presented in this review as powerful tools for the synthesis of functionalized molecules containing heteroatoms.
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Recent progress in the development of fluorometric and colorimetric chemosensors for detection of cyanide ions

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C4CS00008K, Tutorial ReviewFang Wang, Li Wang, Xiaoqiang Chen, Juyoung Yoon
In this review, recent advances made in the development of fluorometric and colorimetric sensors for cyanide anions are highlighted.
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Zeolitic imidazolate framework composite membranes and thin films: synthesis and applications

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C3CS60480B, Review ArticleJianfeng Yao, Huanting Wang
The recent developments of zeolitic imidazolate framework (ZIF) membranes/films, ZIF-polymer mixed matrix membranes and their applications are reviewed in this article.
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Tantalum-based semiconductors for solar water splitting

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, Advance Article
DOI: 10.1039/C3CS60438A, Review ArticlePeng Zhang, Jijie Zhang, Jinlong Gong
This review describes the current status of the design, synthesis, and applications of tantalum-based semiconductors, including tantalum oxides, tantalates and tantalum (oxy)nitrides, for photocatalytic and photoelectrochemical water splitting.
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Phosphine catalysis of allenes with electrophiles

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,2927-2940
DOI: 10.1039/C4CS00054D, Tutorial ReviewZhiming Wang, Xingzhu Xu, Ohyun Kwon
This article compiles the most representative examples of phosphine-catalyzed annulations between allenes and electrophiles to form various carbo- and heterocycles.
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The conversion of allenes to strained three-membered heterocycles

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,3136-3163
DOI: 10.1039/C3CS60416K, Review ArticleC. S. Adams, C. D. Weatherly, E. G. Burke, J. M. Schomaker
The addition of heteroatoms to an allenic double bond yields strained heterocycles that serve as scaffolds for further useful transformations.
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Electrophilic activation of allenenes and allenynes: analogies and differences between Bronsted and Lewis acid activation

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,2916-2926
DOI: 10.1039/C4CS00023D, Tutorial ReviewT. Caneque, F. M. Truscott, R. Rodriguez, G. Maestri, M. Malacria
This review focuses on electrophilic activation of allenes by an acid. Key mechanistic features are presented together with recent synthetic applications.
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[4+2] and [4+3] catalytic cycloadditions of allenes

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,2904-2915
DOI: 10.1039/C4CS00024B, Tutorial ReviewFernando Lopez, Jose L. Mascarenas
This review summarizes the different catalytic [4+2] and [4+3] cycloadditions that have been developed by using allenes as 2C, 3C or even 4C atom partners.
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Cyclization reactions of bis(allenes) for the synthesis of polycarbo(hetero)cycles

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,3106-3135
DOI: 10.1039/C3CS60462D, Review ArticleBenito Alcaide, Pedro Almendros, Cristina Aragoncillo
This review presents the reactivity of a variety of substituted bis(allenes) under different reaction conditions, showing the high number of complex structures that can be obtained.
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Allenes and computational chemistry: from bonding situations to reaction mechanisms

19 April, 2014 - 11:54

Chem. Soc. Rev., 2014, 43,3041-3105
DOI: 10.1039/C3CS60457H, Review ArticleElena Soriano, Israel Fernandez
This review covers the state-of-the-art applications of computational chemistry to understand and rationalize the bonding situation and vast reactivity of allenes.
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