Chem. Soc. Rev.

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Spectroscopy of single nanocrystals

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1311-1337
DOI: 10.1039/C3CS60209E, Review ArticleMark J. Fernee, Philippe Tamarat, Brahim Lounis
Spectroscopic studies of single nanocrystals have been instrumental in unraveling their complex photo-physics.
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Single molecule methods for the study of catalysis: from enzymes to heterogeneous catalysts

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,990-1006
DOI: 10.1039/C3CS60245A, Tutorial ReviewKris P. F. Janssen, Gert De Cremer, Robert K. Neely, Alexey V. Kubarev, Jordi Van Loon, Johan A. Martens, Dirk E. De Vos, Maarten B. J. Roeffaers, Johan Hofkens
Single molecule fluorescence microscopy allows experimental access to the world of catalysts at the nanoscale, providing unique insights.
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Forster resonance energy transfer and kinesin motor proteins

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1144-1155
DOI: 10.1039/C3CS60292C, Review ArticleBram Prevo, Erwin J. G. Peterman
This review highlights the application of FRET to kinesin motor proteins to study how conformational changes underlie function.
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Fluorescent proteins for live-cell imaging with super-resolution

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1088-1106
DOI: 10.1039/C3CS60171D, Review ArticleKarin Nienhaus, G. Ulrich Nienhaus
Photoactivatable fluorescent proteins are key tools for live-cell imaging with high spatial and temporal resolution.
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Spatiotemporal catalytic dynamics within single nanocatalysts revealed by single-molecule microscopy

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1107-1117
DOI: 10.1039/C3CS60215J, Review ArticlePeng Chen, Xiaochun Zhou, Nesha May Andoy, Kyu-Sung Han, Eric Choudhary, Ningmu Zou, Guanqun Chen, Hao Shen
Single-molecule super-resolution fluorescence microscopy uncovers temporal catalytic dynamics and spatial activity patterns within single catalyst nanoparticles.
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Alternating-laser excitation: single-molecule FRET and beyond

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1156-1171
DOI: 10.1039/C3CS60233H, Review ArticleJohannes Hohlbein, Timothy D. Craggs, Thorben Cordes
We discuss the concept behind the alternating-laser excitation scheme, which continues to expand the possibilities of fluorescence-based assays to study biological entities and interactions.
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Breaking the concentration limit of optical single-molecule detection

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1014-1028
DOI: 10.1039/C3CS60207A, Tutorial ReviewPhil Holzmeister, Guillermo P. Acuna, Dina Grohmann, Philip Tinnefeld
Recent optical single-molecule detection methods expand the detection towards the biologically and diagnostically relevant concentration range.
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Molecular plasmonics for nanoscale spectroscopy

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1230-1247
DOI: 10.1039/C3CS60187K, Review ArticleMatthew D. Sonntag, Jordan M. Klingsporn, Alyssa B. Zrimsek, Bhavya Sharma, Laura K. Ruvuna, Richard P. Van Duyne
Single-molecule/single-particle Raman and LSPR spectroscopies advance the fundamental understanding of the interactions between light and matter.
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Maximizing information content of single-molecule FRET experiments: multi-color FRET and FRET combined with force or torque

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1007-1013
DOI: 10.1039/C3CS60184F, Tutorial ReviewSungchul Hohng, Sanghwa Lee, Jinwoo Lee, Myung Hyun Jo
Single-molecule multi-color FRET and single-molecule FRET combined with force or torque.
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Visualizing cellular machines with colocalization single molecule microscopy

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1189-1200
DOI: 10.1039/C3CS60208G, Review ArticleJoshua D. Larson, Margaret L. Rodgers, Aaron A. Hoskins
Single molecule colocalization microscopy and its application for studying complex biochemical processes are reviewed.
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Single molecule rotational probing of supercooled liquids

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,977-989
DOI: 10.1039/C3CS60186B, Tutorial ReviewKeewook Paeng, Laura J. Kaufman
Recent progress in single molecule rotational measurements of fluorescent probes in supercooled liquids enhances understanding of dynamic heterogeneity in these systems.
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How to switch a fluorophore: from undesired blinking to controlled photoswitching

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1076-1087
DOI: 10.1039/C3CS60195A, Review ArticleSebastian van de Linde, Markus Sauer
Molecular optical photoswitches based on fluorescent proteins and organic dyes are fundamental for super-resolution fluorescence imaging and tracking methods. This review emphasizes the design and development of photoswitches and the requirements they need to fulfill for their successful application in single-molecule localization microscopy.
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Single-molecule optical spectroscopy

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,973-976
DOI: 10.1039/C4CS90001D, EditorialMichel Orrit, Taekjip Ha, Vahid Sandoghdar
Guest editors Michel Orrit, Taekjip Ha and Vahid Sandoghdar introduce the Single-molecule optical spectroscopy themed issue of Chemical Society Reviews.
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DNA replication at the single-molecule level

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1201-1220
DOI: 10.1039/C3CS60391A, Review ArticleS. A. Stratmann, A. M. van Oijen
In this review, we highlight recent progress in single-molecule biophysics research that has led to exciting new findings about the mechanism of DNA replication.
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Enhanced single-molecule spectroscopy in highly confined optical fields: from [small lambda]/2-Fabry-Perot resonators to plasmonic nano-antennas

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1263-1286
DOI: 10.1039/C3CS60357A, Review ArticleAndreas M. Kern, Dai Zhang, Marc Brecht, Alexey I. Chizhik, Antonio Virgilio Failla, Frank Wackenhut, Alfred J. Meixner
We review the enhancement of single molecule emission by modifying the optical density of states using plasmonic nanostructures and microresonators.
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Shedding light on protein folding landscapes by single-molecule fluorescence

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1172-1188
DOI: 10.1039/C3CS60311C, Review ArticlePriya R. Banerjee, Ashok A. Deniz
This review presents the efficacy and promise of single-molecule fluorescence methods in studying protein folding, misfolding and aggregation.
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Sizing up single-molecule enzymatic conformational dynamics

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1118-1143
DOI: 10.1039/C3CS60191A, Review ArticleH. Peter Lu
Enzymatic reactions and related protein conformational dynamics are complex and inhomogeneous, playing crucial roles in biological functions.
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Deconstructing the photon stream from single nanocrystals: from binning to correlation

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1287-1310
DOI: 10.1039/C3CS60330J, Review ArticleJian Cui, Andrew P. Beyler, Thomas S. Bischof, Mark W. B. Wilson, Moungi G. Bawendi
We review how different paradigms for deconstructing the photon stream from single nanocrystals have advanced our understanding of their photophysics.
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Single-molecule photophysics, from cryogenic to ambient conditions

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1029-1043
DOI: 10.1039/C3CS60165J, Review ArticleBoleslaw Kozankiewicz, Michel Orrit
Photophysics of the triplet states, new systems and effects connected with spectral diffusion and charge transfer are discussed on the basis of single-molecule experiments.
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Ultra-stable organic fluorophores for single-molecule research

23 February, 2014 - 22:54

Chem. Soc. Rev., 2014, 43,1044-1056
DOI: 10.1039/C3CS60237K, Review ArticleQinsi Zheng, Manuel F. Juette, Steffen Jockusch, Michael R. Wasserman, Zhou Zhou, Roger B. Altman, Scott C. Blanchard
Important strides toward the development of "ultra-stable" fluorophores are reviewed in the context of new frontiers in single-molecule imaging.
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