Dalton Transactions

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Carbon Monoxide Release Properties and Molecular Structures of Thiophenolatomanganese(I) Carbonyl Complexes of the Type [(OC)4Mn([small micro]-S-Aryl)]2 (Mn-based CORMs)

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03567D, PaperMatthias Westerhausen, Ralf Mede, Helmar Gorls, Moritz Klein, Michael Schmitt, J Popp, Vaneza Paola Lorett-Velasquez, Guido Gessner, Stefan H Heinemann
Several phenylthiolatomanganese carbonyl complexes of the type [(OC)4Mn([small micro]-SR)]2 (R = Ph (1a), C6H4-4-CH3 (1b), C6H4-4-CF3 (1c), C6H4-4-F (1d), C6H4-4-Cl (1e), C6H4-4-OMe (1f), C6F5 (1g), and CH2C6H4-4-Cl (1h)) have been prepared...
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Thermoelectric efficiency of (1 x)(GeTe) x(Bi2Se0.2Te2.8) and implementation into highly performing thermoelectric power generators

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03425B, PaperJan Daniel Konig, Markus Winkler, Torben Dankwort, Anna Lena Hansen, Hans Fridtjof Pernau, Viola Duppel, Martin Jaegle, Kilian Bartholome, Lorenz Kienle, Wolfgang Bensch
Here we report for the first time on a complete simulation assisted "material to module" development of a high performance thermoelectric generator (TEG) based on the combination of a phase...
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Binary Lanthanide(III)/Nitrate and Ternary Lanthanide(III)/Nitrate/Chloride Complexes in an Ionic Liquid Containing Water: Optical Absorption and Luminescence Studies

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03479A, PaperSeraj Ansari, Lisheng Liu, Linfeng Rao
This is an Accepted Manuscript, which has been through the RSC Publishing peer review process and has been accepted for publication. Accepted manuscripts are published online shortly after acceptance. This version of the article will be replaced by the fully edited, formatted and proof read Advance Article as soon as this is available.
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Assembly of Silver Alkynyl Compounds with Various Nuclearities

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03394A, PaperYu-Mei Lin, Zong-Jie Guan, Kuan-Guan Liu, Zhanguo Jiang, Quan-Ming Wang
A convenient method for the synthesis of silver alkynyl compounds containing different nuclearities has been developed. The reaction of AgC[identical with]CBut and AgX (X = CF3CO2-, C2F5CO2-) in the presence of...
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Sonochemical synthesis of Au nanowires in III-I oxidation state bridged by 4,4[prime or minute]-dicyanamidobiphenyl and application as selective CO gas sensor

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03427A, PaperLeila Tabrizi, Hossein Chiniforoshan
In this research, Au nanowires, gold-containing polymers of the formula [(Au(I)-NCN-R-NCN-Au(III)-NCN-R-NCN-)]n; R: Biphenyl (or NCN-R-NCN: 4,4[prime or minute]-dicyanamidobiphenyl (bpH2)), have been synthesized by sonochemical process. X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS),...
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Tuneable Dynamics of a Scandium Nitride Cluster Inside an Ih-C80 Cage

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT02892A, CommunicationYongqiang Feng, Taishan Wang, Junfeng Xiang, Li-Hua Gan, bo wu, Li Jiang, Chun-Ru Wang
The internal clusters in metallofullerenes usually exhibit certain motion that is potentially usable in molecular gyroscopes and nano-machines. Based on 45Sc NMR, the motion of the scandium nitride cluster within...
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The synthesis of ZnO/SnO2 porous nanofibers for dye adsorption and degradation

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03382E, PaperXiang Chen, Feng Zhang, Qian Wang, Xiao Han, Xin Li, Jiuyu Liu, Huiming Lin, Fengyu Qu
ZnO/SnO2 hetero-nanofibers about 250 nm in diameter and several micrometers in length are synthesized via electrospun method by using zinc chloride and stannous chloride as inorganic source. All fibers are...
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A strategy to enhance efficiency in dye-sensitized solar cells by highly efficient TiO2/ZnS photoanode

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03102D, PaperS Srinivasa Rao, Dinah Punnoose, Ch Venkata Tulasivarma, CH.S.S Pavan Kumar, Chandu V.V.M Gopi, Soo-Kyoung Kim, Heeje Kim
In dye-sensitized solar cells (DSSCs), the TiO2 photoanode film plays an important role in increasing the power conversion efficiency. In this work, TiO2 nanoparticles were first coated on fluorine-doped tin...
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Luminescent Pt(II) Complexes Bearing Dual Isoquinolinyl Pyrazolates: Fundamentals and Applications

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03028A, PaperHsiao Yun Ku, bihai tong, Yun Chi, Hao-Che Kao, Chia-Chi Yeh, Chih-Hao Chang, Gene-Hsiang Lee
A series of four Pt(II) metal complexes with trans-arranged isoquinolinyl azolates have been prepared, [Pt(Lx)2], x = 1 ~ 4, (1 ~ 4). The associated chelates possess various substituents; namely:...
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Reductive Lithium Insertion into B-cation deficient Niobium Perovskite Oxides

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03193H, PaperAntonio Perejon, Michael Andrew Hayward
Reaction between LiH and the AnBn-1O3n cation deficient perovskite phases Ba5Nb4O15, Ba6TiNb4O18 and Ba3LaNb3O12 proceeds by reductive lithium insertion leading to the formation of Ba5LiNb4O15, Ba6LiTiNb4O18 and Ba3LaLiNb3O12 respectively. During...
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Technetium-99m and rhenium-188 complexes with one and two pendant bisphosphonate groups for imaging arterial calcification

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT02965H, PaperPhilip J Blower, Jayanta Kumar Bordoloi, David Berry, Irfan Ullah Khan, Kavitha Sunassee, Rafael T. M. de Rosales, Catherine Shanahan
The first 99mTc and 188Re radiopharmaceuticals containing two pendant bisphosphonate groups has been synthesised, based on the mononuclear M(V) nitride core with two dithiocarbamate ligands each with a pendant bisphosphonate....
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Rhenium and technetium complexes that bind to amyloid-[small beta] plaques

22 December, 2014 - 11:17

Dalton Trans., 2015, Advance Article
DOI: 10.1039/C4DT02969K, PaperDavid J. Hayne, Andrea J. North, Michelle Fodero-Tavoletti, Jonathan M. White, Lin W. Hung, Angela Rigopoulos, Catriona A. McLean, Paul A. Adlard, Uwe Ackermann, Henri Tochon-Danguy, Victor L. Villemagne, Kevin J. Barnham, Paul S. Donnelly
[M(CO)3]+ (M = Tc/Re) complexes with tridentate ligands with a stilbene functional group bind to amyloid-[small beta] plaques associated with Alzheimer's Disease.
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Solid-phase cyclopalladation in S,C,S'-pincer systems: rising alternative to synthesis in solution

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03477E, PaperDiana V. Aleksanyan, Zinaida Klemenkova, Andrey A. Vasil'ev, Arkadii Ya. Gorenberg, Yulia V. Nelyubina, Vladimir A. Kozlov
In pursuit of a new simple approach to complex organometallic systems, a possibility of formation of the palladium-carbon bond in the solid state via direct cyclopalladation has been studied toward...
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Switchable Platinum-based Tweezers with Pt-Pt Bonding and Selective Luminescence Quenching

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03230F, PaperBernold Hasenknopf, Benjamin Doistau, Caroline Rossi-Gendron, Arnaud Tron, Nathan D McClenaghan, Lise-Marie Chamoreau, Guillaume Vives
Molecular tweezers incorporating peripheral platinum salphen complexes and a central chelating terpyridine group have been synthesized. The terpyridine can be switched upon metal binding between a free 'W' shaped form...
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Three new solvent-directed Cd(II)-based MOFs with unique luminescent properties and highly selective sensor for Cu2+ cations and nitrobenzene

22 December, 2014 - 11:17
Dalton Trans., 2014, Accepted Manuscript
DOI: 10.1039/C4DT03415E, PaperYao-Yu Wang, Guo-Ping Yang, Yun-Long Wu
Three new solvent-induced metal-organic frameworks (MOFs), [Cd(H2L)(H2O)3][round bullet, filled]NMP (1), [Cd3(L)(H2O)4(OH)2] (2) and [Cd(L)0.5(H2O)2][round bullet, filled]H2O (3), have been rationally designed and successfully prepared via solvothermal reaction by the multidentate phenyltetracarboxylic acid [1,1':4',1''-terphenyl]-2',3,3'',5'-tetracarboxylic acid...
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A fluoride bridged {CrIII4DyIII4} single molecule magnet

22 December, 2014 - 11:17

Dalton Trans., 2015, 44,912-915
DOI: 10.1039/C4DT03100H, CommunicationStuart K. Langley, Craig M. Forsyth, Boujemaa Moubaraki, Keith S. Murray
Fluoride bridging between DyDy neighbours in an octanuclear {CrIII4DyIII4} cluster of the 'square-in-square' structural type is the key reason for enhanced single molecule magnetic properties of Cr-Dy SMMs and, particularly, when compared to a reported azido bridged {CrIII4DyIII4} structural analogue.
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Synthesis of aromatic functionalized cage-rearranged silsesquioxanes (T8, T10, and T12) via nucleophilic substitution reactions

22 December, 2014 - 11:17

Dalton Trans., 2015, 44,916-919
DOI: 10.1039/C4DT02941K, CommunicationSupansa Chimjarn, Rungthip Kunthom, Prapassorn Chancharone, Rapheepraew Sodkhomkhum, Preeyanuch Sangtrirutnugul, Vuthichai Ervithayasuporn
Organic-inorganic hybrid nano-building blocks of aryl nitro-, aldehyde-, and bromo-functionalized polyhedral oligomeric silsesquioxanes (T8, T10, and T12) were easily prepared through nucleophilic substitutions.
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[RuV(NCN-Me)(bpy)([double bond, length as m-dash]O)]3+ Mediates efficient C-H bond oxidation from NADH analogs in aqueous media rather than water oxidation

22 December, 2014 - 11:17

Dalton Trans., 2015, 44,920-923
DOI: 10.1039/C4DT02827A, CommunicationJully Patel, Karunamay Majee, Ejaz Ahmạd, Koji Tanaka, Sumanta Kumar Padhi
The [RuV[double bond, length as m-dash]O]3+ and [RuVI[double bond, length as m-dash]O]4+ generated from [RuII(NCN-Me)(bpy)(H2O)](PF6)2 play the selective role in C-H bond oxidation of 2-(pyridin-2-yl)-9,10-dihydroacridine (PADHH) and water splitting, respectively, are reported.
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Four-coordinate Co(II) and Fe(II) complexes with bis(N-heterocyclic carbene)borate and their magnetic properties

22 December, 2014 - 11:17

Dalton Trans., 2015, 44,908-911
DOI: 10.1039/C4DT02537G, CommunicationYuan-Zhong Liu, Jing Wang, Yue Zhao, Lei Chen, Xue-Tai Chen, Zi-Ling Xue
Both square planar and tetrahedral isomers of the four-coordinate Co(II) complex with a bis(N-heterocyclic carbene)borate ligand were isolated while only a tetrahedral configuration was found for the Fe(II) analogue.
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Assembly of a M4L4 "folded-cube" using a T-shaped, right-angled ligand

22 December, 2014 - 11:17

Dalton Trans., 2015, 44,898-902
DOI: 10.1039/C4DT03198A, CommunicationIsmail Elguraish, Kelong Zhu, Leslie A. Hernandez, Hazem Amarne, Jingwei Luo, V. Nicholas Vukotic, Stephen J. Loeb
A new bipyridine ligand based on a T-shaped 2,4,7-trisubstituted benzimidazole framework was synthesised. When combined with [Pt(dppp)]2+ corners, eight right angles (four metal and four ligand) combine to form a M4L4 cluster with an unusual folded-cube structure.
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