Royal Society of Chemistry

Efficient asymmetric synthesis of spiro-2(3H)-furanones via phase-transfer-catalyzed alkynylation

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5388-5392
DOI: 10.1039/C4OB00969J, PaperXiangfei Wu, Seiji Shirakawa, Keiji Maruoka
Efficient asymmetric synthesis of spiro-2(3H)-furanones was achieved via chiral phase-transfer-catalyzed alkynylation.
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Tuning of the HOMO-LUMO gap of donor-substituted symmetrical and unsymmetrical benzothiadiazoles

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5448-5457
DOI: 10.1039/C4OB00629A, PaperRajneesh Misra, Prabhat Gautam
This article reports the design and synthesis of donor-substituted symmetrical and unsymmetrical benzothiadiazoles (BTDs) 5-12 of type D-[small pi]-A-D, D1-[small pi]-A-D2, D1-A1-A2-D2, D-A1-A2-D and D-A1-A2-A1-D by Ullmann, Suzuki and cycloaddition-retroelectrocyclization reactions.
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Efficient C(sp3alkyl)-SCF3 bond formations via copper-mediated trifluoromethylthiolation of alkyl halides

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5500-5508
DOI: 10.1039/C4OB00403E, PaperQuanfu Lin, Li Chen, Yangjie Huang, Mingguang Rong, Yaofeng Yuan, Zhiqiang Weng
An efficient synthesis of alkyl trifluoromethyl sulfides via copper-mediated trifluoromethylthiolation of primary and secondary alkyl halides was described.
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Design, synthesis, and fungicidal activity of novel carboxylic acid amides represented by N-benzhydryl valinamode carbamates

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5427-5434
DOI: 10.1039/C4OB00744A, PaperXiu-Jiang Du, Qiang Bian, Hong-Xue Wang, Shu-Jing Yu, Jun-Jie Kou, Zhi-Peng Wang, Zheng-Ming Li, Wei-Guang Zhao
A series of valinamide carbamate derivatives were designed and synthesized by introducing substituted aromatic rings into valinamide carbamate leads. Bioassays showed that some title compounds exhibited very good fungicidal activity.
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An intracellularly activatable, fluorogenic probe for cancer imaging

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5365-5374
DOI: 10.1039/C4OB00297K, PaperRuisong Tian, Mingjie Li, Jin Wang, Min Yu, Xiuqi Kong, Yupeng Feng, Zeming Chen, Yuxi Li, Weiqiang Huang, Wenjie Wu, Zhangyong Hong
A newly designed, dual-functional probe based on intracellular activation has been successfully developed for the detection of cancer cells.
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The metal tin promoted cascade reaction of ketones in aqueous media for the construction of 2-bromo-4-aryl-1,3-pentadiene

Org. and Biomol. Chem. - 7 July, 2014 - 05:54

Org. Biomol. Chem., 2014, 12,5393-5399
DOI: 10.1039/C4OB00584H, PaperLingyan Liu, Yan Zhang, Hua Zhang, Kaimeng Huang, Bo-xin Gao, Min Zou, Xin Zhou, Hongkai Wang, Jing Li
A novel Barbier-type allenylation cascade reaction of carbonyl compounds promoted by tin was discovered, and afforded a new, highly functionalized 1,3-pentadiene.
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Recent developments of direct rhenium-catalyzed [1,3]-transpositions of allylic alcohols and their silyl ethers

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4381-4394
DOI: 10.1039/C4CS00036F, Tutorial ReviewIvan Volchkov, Daesung Lee
This tutorial review describes recent developments of various allylic transposition strategies involving rhenium-catalyzed rearrangement followed by regio- and stereostereoselective trapping processes and their applications to natural product synthesis.
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The OPEP protein model: from single molecules, amyloid formation, crowding and hydrodynamics to DNA/RNA systems

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4871-4893
DOI: 10.1039/C4CS00048J, Review ArticleFabio Sterpone, Simone Melchionna, Pierre Tuffery, Samuela Pasquali, Normand Mousseau, Tristan Cragnolini, Yassmine Chebaro, Jean-Francois St-Pierre, Maria Kalimeri, Alessandro Barducci, Yoann Laurin, Alex Tek, Marc Baaden, Phuong Hoang Nguyen, Philippe Derreumaux
The OPEP coarse-grained protein model has been applied to a wide range of applications since its first release 15 years ago.
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Chemical sensing of neurotransmitters

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4684-4713
DOI: 10.1039/C3CS60477B, Review ArticleTuhin Pradhan, Hyo Sung Jung, Joo Hee Jang, Tae Woo Kim, Chulhun Kang, Jong Seung Kim
This review focuses on the chemosensors for neurotransmitters published for the last 12 years, covering biogenic amines (dopamine, epinephrine, norepinephrine, serotonin, histamine and acetylcholine), amino acids (glutamate, aspartate, GABA, glycine and tyrosine), and adenosine.
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Catalytic bismetallative multicomponent coupling reactions: scope, applications, and mechanisms

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4368-4380
DOI: 10.1039/C3CS60482A, Tutorial ReviewHee Yeon Cho, James P. Morken
This review covers the bis-metallative coupling of unsaturated functional groups under the agency of transition metal catalysts.
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Structural modification strategies for the rational design of red/NIR region BODIPYs

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4778-4823
DOI: 10.1039/C4CS00030G, Review ArticleHua Lu, John Mack, Yongchao Yang, Zhen Shen
The structure-property relationships of red/NIR region BODIPY dyes is analyzed, so that trends in their photophysical properties can be readily compared.
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AIE macromolecules: syntheses, structures and functionalities

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4494-4562
DOI: 10.1039/C4CS00044G, Review ArticleRongrong Hu, Nelson L. C. Leung, Ben Zhong Tang
A comprehensive review of macromolecules with aggregation-induced emission attributes is presented, covering the frontiers of syntheses, structures, functionalities and applications.
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Atomistic simulation of transport phenomena in nanoelectronic devices

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4357-4367
DOI: 10.1039/C4CS00084F, Tutorial ReviewMathieu Luisier
This paper presents a sophisticated approach to treat quantum transport in nanostructures, covering the basic equations up to relevant applications.
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Anti-cancer palladium complexes: a focus on PdX2L2, palladacycles and related complexes

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4751-4777
DOI: 10.1039/C4CS00063C, Review ArticleAnant R. Kapdi, Ian J. S. Fairlamb
Much success has been achieved with platinum-based chemotherapeutic agents, i.e. through interactions with DNA. The long-term application of Pt complexes is thwarted by issues, leading scientists to examine other metals such as palladium which could exhibit complementary modes of action.
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Macro-/micro-environment-sensitive chemosensing and biological imaging

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4563-4601
DOI: 10.1039/C4CS00051J, Review ArticleZhigang Yang, Jianfang Cao, Yanxia He, Jung Ho Yang, Taeyoung Kim, Xiaojun Peng, Jong Seung Kim
We have summarized the research progress on fluorescent sensors responsive to environmental factors, including local viscosity, polarity, temperature, hypoxia and pH.
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Applications of Bartoli indole synthesis

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4728-4750
DOI: 10.1039/C4CS00045E, Review ArticleGiuseppe Bartoli, Renato Dalpozzo, Monica Nardi
Bartoli indole synthesis is the reaction of choice for the synthesis of many biologically interesting 7-substituted indoles.
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Porous carbon spheres and monoliths: morphology control, pore size tuning and their applications as Li-ion battery anode materials

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4341-4356
DOI: 10.1039/C4CS00071D, Tutorial ReviewAled D. Roberts, Xu Li, Haifei Zhang
Various synthetic techniques are employed to fabricate porous carbon spheres and monoliths for improved performance as Li-ion battery anode materials.
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Organic nanophotonics: from controllable assembly of functional molecules to low-dimensional materials with desired photonic properties

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4325-4340
DOI: 10.1039/C4CS00098F, Tutorial ReviewYongli Yan, Yong Sheng Zhao
The tutorial review aims to provide an insight into the relationship among opto-functional molecules, controllable assembly, diverse nanostructures and photonic properties, which can further guide the function-oriented design and synthesis of low-dimensional materials for integrated photonic devices.
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Nanoparticles meet electrospinning: recent advances and future prospects

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4423-4448
DOI: 10.1039/C3CS60426H, Review ArticleChuan-Ling Zhang, Shu-Hong Yu
In this critical review, the latest advances on nanoparticles-electrospun fibres by post-treatment of the as-prepared electrospun fibres or directly adding nanoparticles into electrospun solution have been overviewed. The application potentials of the nanoparticle-electrospun fibre composites and the trends in this emerging field have been described.
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Structure of organic solids at low temperature and high pressure

Chem. Soc. Rev. - 7 July, 2014 - 05:54

Chem. Soc. Rev., 2014, 43,4300-4311
DOI: 10.1039/C4CS00046C, Tutorial ReviewRachael Lee, Judith A. K. Howard, Michael R. Probert, Jonathan W. Steed
This tutorial review summarises the current state of the art in low temperature and high pressure crystallography of molecular organic and coordination compounds.
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